Gd@C60-based MRI contrast agents

COLL 215

Robert D. Bolskar, bolskar@tda.com1, James W. Raebiger, jraebiger@tda.com1, Juliette R. Petersen, jpetersen@tda.com1, Balaji Sitharaman, balu@rice.edu2, and Lon J. Wilson, durango@rice.edu2. (1) TDA Research, Inc, 12345 West 52nd Avenue, Wheat Ridge, CO 80033, (2) Department of Chemistry and the Richard E. Smalley Institute for Nanoscale Science and Technology, Rice University, Houston, TX 77005
Endohedral metallofullerenes encapsulating Gd are a promising new class of magnetic resonance imaging (MRI) contrast enhancing agents. They offer a safe contrast agent platform lacking the potential for free Gd3+ toxicity due to the very high stability of endohedral Gd sequestration, which is not compromised under physiological conditions. We have developed means to produce, separate and derivatize Gd@C60 molecules for contrast agent applications. Gd@C60 materials water-solubilized with carboxylate and hydroxyl functionalities are effective T1 MR imaging agents with r1 relaxivities higher than current clinically used Gd chelate agents. Using a combination of techniques, including light-scattering, cryo-TEM and NMRD analyses, we have characterized the Gd@C60 derivatives' intermolecular aggregation properties in correlation with their aqueous relaxivity properties. An overview of our ongoing studies of these interesting materials will be presented.
 

Advances in Nanomedicine
1:30 PM-5:20 PM, Monday, 11 September 2006 Sir Francis Drake -- Monterey/Cypress Rooms, Oral

Division of Colloid & Surface Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006