Silk regeneration with ionic liquids

I&EC 178

David M. Phillips, david.phillips@wpafb.af.mil, Air Force Research Laboratory, Materials and Manufacturing Directorate, AFRL Wright-Patterson Air Force Base, 3005 Hobson Way, Wright-Patterson Air Force Base, Dayton, OH 45433, Lawrence F. Drummy, lawrence.drummy@wpafb.af.mil, UES, Inc, Dayton, OH 45432, Rajesh R. Naik, Rajesh.Naik@wpafb.af.mil, Materials and Manufacturing Directorate, Air Force Research Laboratory, 3005 Hobson Way, Bldg 651, R-197, Wright-Patterson AFB, OH 45433-7707, Paul C. Trulove, trulove@usna.edu, Department of Chemistry, United States Naval Academy, 572M Holloway Rd, Stop 9B, Annapolis, MD 21402-5026, Hugh C. De Long, Directorate of Chemistry and Life Sciences, Air Force Office of Scientific Research, 875 North Randolph Street, Suite 325, Room 3112, Arlington, VA 22203-1768, and Robert A. Mantz, robert.mantz@wpafb.af.mil, AFRL/MLBT, Air Force Research Laboratory, Wright Patterson Air Force Base, Ohio, Bldg. 654, Rm 136, 2941 P Street, Wright Patterson AFB, OH 45433.
The properties of silk from the silkworm Bombyx mori are quite remarkable considering that the silkworm processes its silk at ambient conditions in an aqueous solution and the mechanical properties of the silk rival synthetic materials that are processed using organic solvents under harsh conditions.[1] We are exploring alternative processing methodologies for silk that will possibly expand its applications.

It has been shown previously that dialkyl- and trialkylimidazolium based ionic liquids can directly dissolve silkworm cocoon silk to form stable solutions in contrast to other dissolution methods that require a time-intensive, multi step process.[2] These ionic liquid silk solutions have been used to generate both films [2] and fibers.[3] In this work, we further examine the processing conditions required to produce silk fibers from ionic liquid solutions.

[1] D.L. Kaplan, S.J. Lombardi, W. Muller, S. Fossey, in Biomaterials from Biological Sources (Ed: D. Byrom), Stockton Press, New York 1991. [2] D.M. Phillips, L.F. Drummy, D.G. Conrady, D.M. Fox, R.R. Naik, M.O. Stone, P.C. Trulove, H.C. De Long, and R.A. Mantz, J. Am. Chem. Soc., 2004, 126(44), 14350-14351.