Peptide-based diversity for diverse organic reactions

ORGN 249

Scott J. Miller, scott.miller@yale.edu, Department of Chemistry, Yale University, 225 Prospect Street, P. O. Box 208107, New Haven, CT 06520-8107
Modern organic synthesis depends heavily on the use of catalysts for selective transformations. We have discovered a class of synthetic peptides that catalyze a number of enantio- and site-selective selective reactions, including group transfers, azide conjugate additions and C-C bond forming processes. This lecture will describe the discovery and use of oligomers containing histidine and thiazolylalanine for various asymmetric bond formations. The connections between peptide sequence and stereoselectivity will be explored in a range of mechanistically distinct reactions. Prospects for generalizations and eventual design of catalysts from first principles will be evaluated.
 

ACS Award in Pure Chemistry
8:00 AM-12:00 PM, Tuesday, 28 March 2006 Georgia World Congress Center -- C303/304/305, Oral

Division of Organic Chemistry

The 231st ACS National Meeting, Atlanta, GA, March 26-30, 2006